Donovan did release a 'Brother Sun, Sister Moon' album in 2004, but it consisted of new rerecordings with just him singing and playing guitar - no orchestra or choir. Apparently he tried to release the original recordings of his songs, but there were complex rights issues over said recordings that he found too difficult to resolve, so he decided to rerecord all the songs and release them that way (though the end credits version of the title track did show up on his 'Newest Bath Guide' single, albeit in a different mix to what you hear in the film). I don't know if these rights issues would still be a problem today, but if Intrada was able to release this soundtrack with all the original Donovan recordings, I'd certainly buy it.
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